Simultaneous Phase Separation and Pattern Formation in Chiral Active Mixtures

Chiral active particles, or self-propelled circle swimmers, from sperm cells to asymmetric Janus colloids, form a rich set of patterns, which are different from those seen in linear swimmers. Such patterns have mainly been explored for identical circle swimmers, while real-world circle swimmers, typically possess a frequency distribution. Here we show that even the simplest mixture of (velocity-aligning) circle swimmers with two different frequencies, hosts a complex world of superstructures: The most remarkable example comprises a microflock pattern, formed in one species, while the other species phase separates and forms a macrocluster, coexisting with a gas phase. Here, one species microphase-separates and selects a characteristic length scale, whereas the other one macrophase separates and selects a density. A second notable example, here occurring in an isotropic system, are patterns comprising two different characteristic length scales, which are controllable via frequency and swimming speed of the individual particles

The Rotating Vicsek Model: Pattern Formation and Enhanced Flocking in Chiral Active Matter

We generalize the Vicsek model to describe the collective behaviour of polar circle swimmers with local alignment interactions. While the phase transition leading to collective motion in 2D (flocking) occurs at the same interaction to noise ratio as for linear swimmers, as we show, circular motion enhances the polarization in the ordered phase (enhanced flocking) and induces secondary instabilities leading to structure formation. Slow rotations result in phase separation whereas fast rotations generate patterns which consist of phase synchronized microflocks of controllable self-limited size. Our results defy the viewpoint that monofrequent rotations form a rather trivial extension of the Vicsek model and establish a generic route to pattern formation in chiral active matter with possible applications to control coarsening and to design rotating microflocks.Comment: Contains a Supplementary Materia

From single-particle to collective effective temperatures in an active fluid of self-propelled particles

We present a comprehensive analysis of effective temperatures based on fluctuation-dissipation relations in a model of an active fluid composed of self-propelled hard disks. We first investigate the relevance of effective temperatures in the dilute and moderately dense fluids. We find that a unique effective temperature does not in general characterize the non-equilibrium dynamics of the active fluid over this broad range of densities, because fluctuation-dissipation relations yield a lengthscale-dependent effective temperature. By contrast, we find that the approach to a non-equilibrium glass transition at very large densities is accompanied by the emergence of a unique effective temperature shared by fluctuations at all lengthscales. This suggests that an effective thermal dynamics generically emerges at long times in very dense suspensions of active particles due to the collective freezing occurring at non-equilibrium glass transitions.Comment: 6 pages, 3 fig

Micro-flock patterns and macro-clusters in chiral active Brownian disks

Chiral active particles (or self-propelled circle swimmers) feature a rich collective behavior, comprising rotating macro-clusters and micro-flock patterns which consist of phase-synchronized rotating clusters with a characteristic self-limited size. These patterns emerge from the competition of alignment interactions and rotations suggesting that they might occur generically in many chiral active matter systems. However, although excluded volume interactions occur naturally among typical circle swimmers, it is not yet clear if macro-clusters and micro-flock patterns survive their presence. The present work shows that both types of pattern do survive but feature strongly enhance fluctuations regarding the size and shape of the individual clusters. Despite these fluctuations, we find that the average micro-flock size still follows the same characteristic scaling law as in the absence of excluded volume interactions, i.e. micro-flock sizes scale linearly with the single-swimmer radius

Synchronization in dynamical networks of locally coupled self-propelled oscillators

Systems of mobile physical entities exchanging information with their neighborhood can be found in many different situations. The understanding of their emergent cooperative behaviour has become an important issue across disciplines, requiring a general conceptual framework in order to harvest the potential of these systems. We study the synchronization of coupled oscillators in time-evolving networks defined by the positions of self-propelled agents interacting in real space. In order to understand the impact of mobility in the synchronization process on general grounds, we introduce a simple model of self-propelled hard disks performing persistent random walks in 2$d$ space and carrying an internal Kuramoto phase oscillator. For non-interacting particles, self-propulsion accelerates synchronization. The competition between agent mobility and excluded volume interactions gives rise to a richer scenario, leading to an optimal self-propulsion speed. We identify two extreme dynamic regimes where synchronization can be understood from theoretical considerations. A systematic analysis of our model quantifies the departure from the latter ideal situations and characterizes the different mechanisms leading the evolution of the system. We show that the synchronization of locally coupled mobile oscillators generically proceeds through coarsening verifying dynamic scaling and sharing strong similarities with the phase ordering dynamics of the 2$d$ XY model following a quench. Our results shed light into the generic mechanisms leading the synchronization of mobile agents, providing a efficient way to understand more complex or specific situations involving time-dependent networks where synchronization, mobility and excluded volume are at play

Velocity alignment promotes motility-induced phase separation

We study the phase behavior of polar Active Brownian Particles moving in two-spatial dimensions and interacting through volume exclusion and velocity alignment. We combine particle-based simulations of the microscopic model with a simple mean-field kinetic model to understand the impact of velocity alignment on the motility-induced phase separation of self-propelled disks. We show that, as the alignment strength is increased, approaching the onset of collective motion from below, orientational correlations grow, rendering the diffusive reorientation dynamics slower. As a consequence, the tendency of particles to aggregate into isotropic clusters is enhanced, favoring the complete de-mixing of the system into a low and high-density phase.Comment: 7 pages, 5 figure

Emergent States in Systems of Chiral Self-Propelled Rods

We study inherently chiral self-propelled particles, self-rotating at a fixed frequency, in two dimensions, subjected to nematic alignment interactions and rotational noise. By means of both, homogeneous and spatially resolved mean field kinetic theory, we identify various different flocking states. We confirm the presence of the predicted phases using agent-based simulations, in particular, an homogeneous nematic phase at low frequencies, followed by a microflock pattern phase at larger frequencies, characterized by finite-size nematic clusters. We emphasize that special care has to be taken within the simulations in order to avoid artifacts, and present a non-standard simulation technique in order to avoid them.Comment: 10 pages, 4 figure